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Research Progress of Cellulose-based Carbon Materials as Oxygen Reduction Reaction Catalysts
Received:May 13, 2025  Revised:June 12, 2025
DOI:10.11980/j.issn.0254-508X.2025.10.016
Key Words:cellulose  carbon materials  catalysts  oxygen reduction reaction
Fund Project:国家自然科学基金(22108137);山东省青年创新团队(2022KJ294);济南市科技局“新高校20条”资助项目自主培养创新团队计划(20233046)。
Author NameAffiliationPostcode
SUN Aoran* State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
ZHANG Zhenzhong State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
JIANG Chengshan State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
ZHANG Lei* State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
YANG Guihua State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
CHEN Jiachuan* State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
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Abstract:In recent years, as the demand for clean-energy technologies continues to rise, conventional Pt-based catalysts are constrained by high cost, resource scarcity, and limited stability, which in turn propels the development of non-precious-metal catalysts. Using abundant, renewable cellulose to prepare porous carbon catalysts offers advantages of low cost, high specific surface area, orderly and tunable porosity, and good chemical stability and conductivity. This review systematically summarized the preparation methods and formation mechanisms of cellulose-based carbon materials, mainly discussed the effects of different approaches including hydrothermal carbonization, chemical/physical activation, hard templating, and aerogel carbonization on structures and properties of cellulose-based carbon materials, reviewed progress in their application to the oxygen reduction reaction (ORR), compared the performances of cellulose-derived carbons with different architectures, and outlined prospects for their research and application in ORR catalysis.
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