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Research Advances in Hydrophobic-Oleophobic Functionalization of Nanocellulose and Its Applications
Received:May 30, 2025  Revised:August 18, 2025
DOI:10.11980/j.issn.0254-508X.2025.10.006
Key Words:nanocellulose  hydrophobic-oleophobic functionalization  bio-based materials
Fund Project:山东省高等学校青年创新团队项目(2023KJ330);全国重点实验室建设重大科研专项(2025ZDGZ02)。
Author NameAffiliationPostcode
FU Bin* State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
ZHOU Rong State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
YAO Yuping Qingdao TGOOD Electric Co., Ltd., Qingdao, Shandong Province, 370200 370200
ZHANG Bo State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
ZHAO Qiaoqiao State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
WANG Shengdan* State Key Lab of Green Papermaking and Resource Recycling, Qilu University of Technology (Shandong Academy of Sciences), Ji’nan, Shandong Province, 250353 250353
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Abstract:As a novel bio-based material, nanocellulose exhibits distinctive attributes including renewability, degradabiility, high specific surface area, and exceptional mechanical performance. However, its surface contains abundant hydrophilic hydroxyl groups, which limits its application in hydrophobic-olephoic fields. Consequently, the hydrophobic-oleophobic functionalization modification of nanocellulose has progressively emerged as a research focus among scientists. In this paper, the principles, methodologies, and applications of hydrophobic-oleophobic functionalization modification of nanocellulose were systematically reviewed, while the characteristic features of products derived from distinct modification approaches were categorized. Applications of hydrophobic-oleophobic modified nanocellulose in food packaging, textile industries, and paper manufacturing were critically evaluated. Technical bottlenecks hindering the scaled application of these materials were analyzed, and future development directions were prospected to provide theoretical foundations for designing high-performance nanocellulose-based hydrophobic-oleophobic systems.
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