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| Preparation of Cellulose/Chitosan Composite Aerogels Loaded with β-FeOOH/Fe3O4 and Degradation Performance of Methyl Orange |
| Received:May 16, 2024 |
| DOI:10.11980/j.issn.0254-508X.2024.12.004 |
| Key Words:cellulose polymorphic iron composite aerogel photocatalysis |
| Fund Project:浙江省“领雁”研发攻关计划项目(2023C03157)。 |
| Author Name | Affiliation | Postcode | | YANG Xiaoyu | Pulp and Papermaking Research Center, College of Textile Science and Engineering, Zhejiang Sci-Tech University, Hangzhou, Zhejiang Province, 310008 | 310018 | | YANG Xiangjian | Pulp and Papermaking Research Center, College of Textile Science and Engineering, Zhejiang Sci-Tech University, Hangzhou, Zhejiang Province, 310008 Zhejiang Huafeng Paper Technology Co., Ltd., Anji, Zhejiang Province, 313309 | 313309 | | LI Feiyun | Pulp and Papermaking Research Center, College of Textile Science and Engineering, Zhejiang Sci-Tech University, Hangzhou, Zhejiang Province, 310008 | 310018 | | CHEN Tianying | Pulp and Papermaking Research Center, College of Textile Science and Engineering, Zhejiang Sci-Tech University, Hangzhou, Zhejiang Province, 310008 | 310018 | | ZOU Xiaofeng | Zhejiang Huafeng Paper Technology Co., Ltd., Anji, Zhejiang Province, 313309 | 313309 | | TANG Yanjun* | Pulp and Papermaking Research Center, College of Textile Science and Engineering, Zhejiang Sci-Tech University, Hangzhou, Zhejiang Province, 310008 | 310018 |
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| Abstract:The study mainly developed the preparation of cellulose/chitosan composite aerogels loaded with visible light catalyst β-FeOOH/Fe3O4, which was subsequently used as a phototropic Fenton-like system to improve the catalytic efficiency. The degradation effect of composite aerogels on methyl orange (MO) with different β-FeOOH/Fe3O4 mass ratios and different loadings was systematically investigated, and the phototropic Fenton-like degradation mechanism was elaborated. The results showed that in phototropic Fenton-like degradation, the degradation rate of MO increased with the increase of loadings. When the mass ratio of β-FeOOH/Fe3O4 was 2∶1, the degradation ability attained the optimum state, with a degradation rate of 89.1%. The results of free radical trapping experiments showed that the main active subtances for photo-induced degradation of methyl orange could be attributed to hydroxyl radicals. |
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