Wang Ruixin1   Zhong Qing2, 3   Xiong Tao3   Lu Siyuan1  Zhou Min1  Li Xinping1  Zhang Zhao1, *
投稿时间:2026-06-08  修订日期:2026-07-27
DOI:
Key Words:Haze Regulation of High-Beating-Degree Pulp/TEMPO-Oxidized Cellulose Nanofiber Composite Transparent Paper and Preliminary Validation as an OLED Substrate
Fund Project:国家自然科学基金项目(22171170;21703131)
作者单位邮编
王睿欣 陕西科技大学 710021
钟清 广致科技荆州有限公司 
熊涛 柯赛科技深圳有限公司 
路思远 陕西科技大学 
周敏 陕西科技大学 
李新平 陕西科技大学 
张召* 陕西科技大学 710021
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Abstract:To explore a paper-based flexible optoelectronic substrate combining light diffusion, surface smoothness, and water-vapor barrier performance, composite transparent paper was prepared from 90°SR high-beating-degree pulp and TEMPO-oxidized cellulose nanofibers (tCNF), followed by single- or double-sided epoxy-resin dip coating. The uncoated samples containing 90°SR pulp exhibited a haze of approximately 94.3%. The single-sided coated sample with a tCNF-to-pulp mass ratio of 1:1 showed a haze of 81.2% and a water-vapor transmission rate of 60.0 g·m?²·d?¹. The double-sided coated samples maintained a transmittance of 86.2%–89.3% and a maximum haze of 58.1%. The double-sided coated 1:1 sample exhibited a root-mean-square roughness of 2.5 nm and a water-vapor transmission rate below the instrumental detection limit (<0.5 g·m?²·d?¹). A representative OLED fabricated on this substrate could be operated and reached a maximum luminance of 15.3 cd·m?² at 18.0 V. The morphological and optical results suggest that microscale fibers, fiber bundles, and air/cellulose interfaces act as important scattering structures, whereas double-sided coating improves surface smoothness and barrier performance by sealing connected pores. This study provides a preliminary proof of concept for constructing a paper-based light-diffusing OLED substrate, while the independent effect of coating amount and device reproducibility require further evaluation.
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